Jewett, SL, Olmsted,
HK, Marach, JA,
Rojas,
F, and Silva KE
(2000). Anion Protection of CuZnSOD During Peroxidative Activity
with H2O2 (Peroxidase Activity of CuZn SOD:
A Misnomer. Biochem. Biophys. Res. Commun. 274:
57-60 (PDF file available on request sandra.jewett@csun.edu)
ABSTRACT
The peroxidase activity of the copper-zinc superoxide
dismutase is a poorly sustained activity because of the competing inactivation
of the enzyme. New evidence suggests that the bound oxidant
may be partitioning between oxidizing the enzyme or oxidizing small anions.
At constant peroxide, nitrite and azide only partially protect the enzyme
(50%) against loss of copper(I) and inactivation up to one anion per copper.
Beyond that level, there is no further protection. Bicarbonate ion
also protects but larger amounts are required. These data suggest
that there is significant oxidation of the enzyme even in the presence
of the small anions and therefore the formation of the bound oxidant cannot
be sustained in a true catalytic process.